Christian Wäckerlin
Mission
Our mission is to explore electronic transport through low-dimensional (1D and 2D) metal-organic nanomaterials from a basic science perspective. We want to obtain a fundamental understanding of their geometrical and electronic structure and their magnetic properties to ultimately exploit our new knowledge towards prototype devices.
We synthesize the low-dimensional metal-organic nanomaterials by chemical reaction of metal atoms and precursor molecules directly at surfaces in ultra-high-vacuum. In order to characterize and understand their formation, electronic properties and in particular their electronic conductivity, we combine low-temperature scanning probe microscopy (STM/nc-AFM) with photoelectron spectroscopy (XPS, UPS) and X-ray absorption spectroscopy/X-ray magnetic circular dichroism (XAS/XMCD). We also employ a unique in-situ variant of time-of-flight mass spectrometry (ToF-SIMS) as a method for the extremely precise analytics of our nanomaterials.
Awards
SNSF Eccellenza Professorial Fellowship
Swiss National Science Foundation
2021
Selected publications
On-Surface Hydrogen/Deuterium Isotope Exchange in Polycyclic Aromatic Hydrocarbons
C. Wäckerlin
Published in Angewandte Chemie, 2021, 60, 8446–8449 in
On-Surface Hydrogenation of Buckybowls: From Curved Aromatic Molecules to Planar Non-Kekulé Aromatic Hydrocarbons
C. Wäckerlin, A. Gallardo, A. Mairena, M. Baljozović, A. CahlÃk, A. AntalÃk, J. Brabec, L. Veis, D. Nachtigallová, P. JelÃnek, K.-H. Ernst
Published in ACS Nano, 2020, 14, 16735−16742 in
Magnetic remanence in single atoms
F. Donati, S. Rusponi, S. Stepanow, C. Wäckerlin, A. Singha, L. Persichetti, R. Baltic, K. Diller, F. Patthey, E. Fernandes, J. Dreiser, Ž. Å ljivanÄanin, K. Kummer, C. Nistor, P. Gambardella, H. Brune
Published in Science, 2016, 352, 318–321 in
Ranking the Stability of Transition Metal Complexes by On-Surface Atom Exchange
A. Rieger, S. Schnidrig, B. Probst, K.-H. Ernst, C. Wäckerlin
Published in The Journal of Physical Chemistry Letters in
Giant Hysteresis of Single-Molecule Magnets Adsorbed on a Nonmagnetic Insulator
C. Wäckerlin, F. Donati, A. Singha, R. Baltic, S. Rusponi, K. Diller, F. Patthey, M. Pivetta, Y. Lan, S. Klyatskaya, M. Ruben, H. Brune, J. Dreiser
Published in Advanced Materials, 2016, 28, 5195–5199 in
Ammonia Coordination Introducing a Magnetic Moment in On-Surface Low-Spin Porphyrin
C. Wäckerlin, K. Tarafder, J. Girovsky, J. Nowakowski, T. Hählen, A. Shchyrba, D. Siewert, A. Kleibert, F. Nolting, P. M. Oppeneer, T. A. Jung, N. Ballav
Published in Angewandte Chemie International Edition, 2013, 52, 4568–4571 in
Controlling spins in adsorbed molecules by a chemical switch
C. Wäckerlin, D. Chylarecka, A. Kleibert, K. Müller, C. Iacovita, F. Nolting, T. A. Jung, N. Ballav
Published in Nature Communications, 2010, 1, 61 in
Teaching & PhD
PhD Students
Quy Hien Le, Diego Radillo Ochoa, Céline Hensky
Courses
Physics of low-dimensional materials
PHYS-474
This course covers the concepts and physics of matter at reduced dimensions. The fabrication and characterization of low-dimensional materials as well as their potential application is discussed. The critical review and presentation of scientific publications is trained.