Christian Wäckerlin

EPFL SB IPHYS GR-CW
PH A1 365 (Bâtiment PH)
Station 3
1015 Lausanne

Mission

In the future, the global society will even critically rely on systems for information and communications technology. We will want to perform more operations (data storage, signal transmission, and computation) faster, with less energy and on devices involving fewer atoms.
Our mission is to explore electronic transport through low-dimensional (1D and 2D) metal-organic nanomaterials from a basic science perspective. We want to obtain a fundamental understanding of their geometrical and electronic structure and their magnetic properties to ultimately exploit our new knowledge towards prototype devices.
We synthesize the low-dimensional metal-organic nanomaterials by chemical reaction of metal atoms and precursor molecules directly at surfaces in ultra-high-vacuum. In order to characterize and understand their formation, electronic properties and in particular their electronic conductivity, we combine low-temperature scanning probe microscopy (STM/nc-AFM) with photoelectron spectroscopy (XPS, UPS) and X-ray absorption spectroscopy/X-ray magnetic circular dichroism (XAS/XMCD). We also employ a unique in-situ variant of time-of-flight mass spectrometry (ToF-SIMS) as a method for the extremely precise analytics of our nanomaterials.

Awards

SNSF Eccellenza Professorial Fellowship

Swiss National Science Foundation

2021

Selected publications

On-Surface Hydrogen/Deuterium Isotope Exchange in Polycyclic Aromatic Hydrocarbons

C. Wäckerlin
Published in Angewandte Chemie, 2021, 60, 8446–8449 in

On-Surface Hydrogenation of Buckybowls: From Curved Aromatic Molecules to Planar Non-Kekulé Aromatic Hydrocarbons

C. Wäckerlin, A. Gallardo, A. Mairena, M. Baljozović, A. Cahlík, A. Antalík, J. Brabec, L. Veis, D. Nachtigallová, P. Jelínek, K.-H. Ernst
Published in ACS Nano, 2020, 14, 16735−16742 in

Magnetic remanence in single atoms

F. Donati, S. Rusponi, S. Stepanow, C. Wäckerlin, A. Singha, L. Persichetti, R. Baltic, K. Diller, F. Patthey, E. Fernandes, J. Dreiser, Ž. Šljivančanin, K. Kummer, C. Nistor, P. Gambardella, H. Brune
Published in Science, 2016, 352, 318–321 in

Ranking the Stability of Transition Metal Complexes by On-Surface Atom Exchange

A. Rieger, S. Schnidrig, B. Probst, K.-H. Ernst, C. Wäckerlin
Published in The Journal of Physical Chemistry Letters in

Giant Hysteresis of Single-Molecule Magnets Adsorbed on a Nonmagnetic Insulator

C. Wäckerlin, F. Donati, A. Singha, R. Baltic, S. Rusponi, K. Diller, F. Patthey, M. Pivetta, Y. Lan, S. Klyatskaya, M. Ruben, H. Brune, J. Dreiser
Published in Advanced Materials, 2016, 28, 5195–5199 in

Ammonia Coordination Introducing a Magnetic Moment in On-Surface Low-Spin Porphyrin

C. Wäckerlin, K. Tarafder, J. Girovsky, J. Nowakowski, T. Hählen, A. Shchyrba, D. Siewert, A. Kleibert, F. Nolting, P. M. Oppeneer, T. A. Jung, N. Ballav
Published in Angewandte Chemie International Edition, 2013, 52, 4568–4571 in

Controlling spins in adsorbed molecules by a chemical switch

C. Wäckerlin, D. Chylarecka, A. Kleibert, K. Müller, C. Iacovita, F. Nolting, T. A. Jung, N. Ballav
Published in Nature Communications, 2010, 1, 61 in

Teaching & PhD

PhD Students

Quy Hien Le, Diego Radillo Ochoa, Céline Hensky

Courses

Physics of low-dimensional materials

PHYS-474

This course covers the concepts and physics of matter at reduced dimensions. The fabrication and characterization of low-dimensional materials as well as their potential application is discussed. The critical review and presentation of scientific publications is trained.